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Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for dark matter. ALP dark matter would manifest as a field oscillating at an (as of yet) unknown frequency. The frequency depends linearly on the ALP mass and plausibly ranges from 10⁻²²to 10 eV/c². This motivates broadband search approaches. We report on a direct search for ALP dark matter with an interferometer composed of two atomic K-Rb-³He comagnetometers, one situated in Mainz, Germany, and the other in Kraków, Poland. We leverage the anticipated spatio-temporal coherence properties of the ALP field and probe all ALP-gradient-spin interactions covering a mass range of nine orders of magnitude. No significant evidence of an ALP signal is found. We thus place new upper limits on the ALP-neutron, ALP-proton and ALP-electron couplings reaching belowg_aNN < 10⁻⁹ GeV⁻¹,g_aPP < 10⁻⁷ GeV⁻¹andg_aee < 10⁻⁶ GeV⁻¹, respectively. These limits improve upon previous laboratory constraints for neutron and proton couplings by up to three orders of magnitude. 

We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741\mathrm{neV}/{\mathrm{c}}^2-5.577733\mathrm{neV}/{\mathrm{c}}^2$by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHZ resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}}\approx 3\times {10}^{-2}{\mathrm{GeV}}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment’s capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\mathrm{peV}/{\mathrm{c}}^2$to $17\mathrm{neV}/{\mathrm{c}}^2$with hyperpolarized samples to boost the sensitivity beyond the astronomical limits. 

Levitated ferromagnets act as ultraprecise magnetometers, which can exhibit high quality factors due to their excellent isolation from the environment. These instruments can be utilized in searches for ultralight dark matter candidates, such as axionlike dark matter or dark-photon dark matter. In addition to being sensitive to an axion-photon coupling or kinetic mixing, which produce physical magnetic fields, ferromagnets are also sensitive to the effective magnetic field (or “axion wind”) produced by an axion-electron coupling. While the dynamics of a levitated ferromagnet in response to a dc magnetic field have been well studied, all of these couplings would produce ac fields. In this work, we study the response of a ferromagnet to an applied ac magnetic field and use these results to project their sensitivity to axion and dark-photon dark matter. We pay special attention to the direction of motion induced by an applied ac field, in particular, whether it precesses around the applied field (similar to an electron spin) or librates in the plane of the field (similar to a compass needle). We show that existing levitated ferromagnet setups can already have comparable sensitivity to an axion-electron coupling as comagnetometer or torsion balance experiments. In addition, future setups can become sensitive probes of axion-electron coupling, dark-photon kinetic mixing, and axion-photon coupling, for ultralight dark matter masses < 5feV.